Question: Consider pure PbO with anion-Frenkel compensation and dominant ionic defects. What are the slopes of the essentially linear dependences in the three limiting regions of

Consider pure PbO with anion-Frenkel compensation and dominant ionic defects. What are the slopes of the essentially linear dependences in the three limiting regions of the plot of defect fractions versus p_O2? Sketch the Brouwer diagram.

Brouwer diagram

VNI h ionic defects dominate reduction [v]= [VNi stoichiometric range oxidation h Ni electronic defects

VNI h ionic defects dominate reduction [v]= [VNI stoichiometric range oxidation h Ni electronic defects dominate reduction [e] = [h*] stoichiometric range h oxidation

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